Data for Manuscript =================== Data for manuscript "Modulated Self-Assembly of Catalytically Active Metal-Organic Nanosheets Containing Zr6 Clusters and Dicarboxylate Ligands” ACS Applied Materials and Interfaces, 2024, 10.1021/acsami.4c00604 Authors: Ram R. R. Prasad, Sophia S. Boyadjieva, Guojun Zhou, Jiangtian Tan, Francesca C. N. Firth, Sanliang Ling, Zhehao Huang, Matthew J. Cliffe, Jonathan A. Foster and Ross S. Forgan Experimental data in Origin format, bruker NMR format and mestrenova files, xrdml powder X-files and as jpg files R. R. R. P. and J. A. F. thank EPSRC (EP/S021124/1) for funding. R. S. F. thanks the Royal Society for receipt of a URF and the University of Glasgow for funding. The work has been supported by the European Research Council (ERC) under the European Union's Horizon 2020 Programme for Research and Innovation (grant agreement no. 677289, SCoTMOF, ERC-2015-STG). Z.H. thanks the Swedish Research Council Formas (2020-00831) and the Swedish Research Council VR (2022-02939) for funding. M. J. C. thanks the School of Chemistry at the University of Nottingham for receipt of a Hobday Fellowship. We acknowledge the use of the ARCHER2 supercomputer through membership of the UK's HPC Materials Chemistry Consortium, which is funded by EPSRC (EP/X035859). CCDC 2314111 contain the supplementary crystallographic data for this paper. These data can be obtained free of charge from The Cambridge Crystallographic Data Centre via www.ccdc.cam.ac.uk/data_request/cif. Data available NMR spectra, Thermogravimetric analysis, powder X-ray diffraction data and refinements, Atomic Force microscopy, SEM images, IR spectra, Catalysis data, and DFT structures